Research Papers: Fuel Combustion

Laser-Induced Plasma Spectrometry With Chemical Seeding and Application to Flow Mixing Analysis in Methane–Air Flames

[+] Author and Article Information
Hirotoshi Taki

Department of Applied Chemistry,
Graduate School of Engineering,
Nagoya University,
Nagoya 464-8603, Japan
e-mail: waterfall.wide.city@hotmail.com

Hiroshi Asai

Department of Applied Chemistry,
Graduate School of Engineering,
Nagoya University,
Nagoya 464-8603, Japan
e-mail: hisroshi@asai.tec.toyota.co.jp

Kuniyuki Kitagawa

EcoTopia Science Institute,
Nagoya University,
Furo-Cho, Chikusa-ku,
Nagoya 464-8603, Japan
e-mail: a41596a@yahoo.co.jp

Hiroyuki Oyama

Advanced Industrial Science
and Technology (AIST),
2-17-2-1, Tsukisamu-Higashi,
Sapporo 062-0051, Japan
e-mail: h.oyama@aist.go.jp

Ashwani K. Gupta

Department of Mechanical Engineering,
University of Maryland,
College Park, MD 20742
e-mail: akgupta@umd.edu

1Corresponding author.

Contributed by the Advanced Energy Systems Division of ASME for publication in the JOURNAL OF ENERGY RESOURCES TECHNOLOGY. Manuscript received May 28, 2014; final manuscript received July 5, 2014; published online July 29, 2014. Editor: Hameed Metghalchi.

J. Energy Resour. Technol 137(1), 012202 (Jul 29, 2014) (5 pages) Paper No: JERT-14-1165; doi: 10.1115/1.4027980 History: Received May 28, 2014; Revised July 05, 2014

Spectroscopic measurements of flames are amongst the most important analytical diagnostic techniques that allow one to improve thermal and energy efficiency of industrial furnaces. A chemical seeding laser-induced plasma spectroscopy (CS-LIPS) was successfully developed and applied for mixing analysis of a methane–air diffusion flame. The results obtained showed that sensitivity of this system was much improved using silica rod as the target material in place of the tungsten material used in our previous studies. Profiling of Mg spectral emission and mixing in the flame was made more clearly with the introduction of magnesium aerosols as a tracer into the combustion air flow.

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Kuprianov, V. I., 2005, “Applications of a Cost-Based Method of Excess Air Optimization for the Improvement of Thermal Efficiency and Environmental Performance of Steam Boilers,” Renewable Sustainable Energy Rev., 9, pp. 474–498. [CrossRef]
Hasegawa, T., Mochida, S., and Gupta, A. K., 2002, “Development of Advanced Industrial Furnace Using Highly Preheated Combustion Air,” J. Propul. Power, 18(2), pp. 233–239. [CrossRef]
Kouprianov, V. I., and Tanetsakunvatana, V., 2003, “Optimization of Excess Air for the Improvement of Environmental Performance for a 150 MW Boiler Fired With Thai Lignite,” Appl. Energy, 74(3/4), pp. 445–453. [CrossRef]
Romero, C., Li, X., Keyvan, S., and Rossow, R., 2005, “Spectrometer-Based Combustion Monitoring for Flame Stoichiometry and Temperature Control,” Appl. Therm. Eng., 25, pp. 659–676. [CrossRef]
Baker, M. R., and Vallee, B. L., 1959, “Theory of Spectral Excitation in Flames as Function of Sample Flow,” Anal. Chem., 31(12), pp. 2036–2039. [CrossRef]
Majd, A. E., Arabanian, A. S., Massudi, R., and Nazeri, M., 2011, “Spatially Resolved Laser-Induced Breakdown Spectroscopy in Methane–Air Diffusion Flames,” Appl. Spectrosc., 65, pp. 36–42. [CrossRef] [PubMed]
Zhang, S., Yu, X., Li, F., Kang, G., Chen, L., and Zhang, X., 2012, “Laser Induced Break-Down Spectroscopy for Local Equivalence Ratio Measurement of Kerosene/Air Mixture at Elevated Pressure,” Opt. Lasers Eng., 50, pp. 877–882. [CrossRef]
Itoh, S., Shinoda, M., Kitagawa, K., Arai, N., Lee, Y. I., Zhao, D., and Yamashita, H., 2001, “Spatially Resolved Elemental Analysis of a Hydrogen–Air Diffusion Flame by Laser-Induced Plasma Spectroscopy (LIPS),” Microchem. J., 70, pp. 143–152. [CrossRef]
Kitagawa, K., Taki, H., and Arai, N., 2002, “Profiling of Elemental Composition in a Methane–Air Premixed Flame by Laser-Induced Plasma Spectroscopy (LIPS),” Energy Convers. Eng. Conf., 37, pp. 382–388.
Shen, Q., Miyata, Y., Morita, S., Baba, Y., Kitagawa, K., and Gupta, A. K., 2013, “Visualization of Two-Dimensional Excitation Temperatures in CH4/N2/Ar Plasmas for Preparation of Carbonaceous Materials,” ASME J. Energy Resour. Technol., 135(3), p. 034501. [CrossRef]
Oyama, H., Kayahana, J., Yatsu, S., Kitagawa, K., and Gupta, A. K., 2014, “Time-Resolved 2D Temperature Measurement From Acetylene-Oxygen Flame Using Chemical Seeding Spectrocamera,” ASME J. Resour. Technol., 136(1), p. 011101. [CrossRef]
Desmira, N., Kitagawa, K., and Gupta, A. K., 2014, “OH and NO Distribution in Mixture of Waste Rice Bran and Octanol Oil Flames,” ASME J. Energy Resour. Technol., 136(1), p. 014501. [CrossRef]
Askari, O., Metghalchi, M., Moghaddas, A., Hannani, S. K., and Ebrahimi, R., 2013, “Fundamental Study of Spray and Partially Premixed Combustion Characteristics of Methane/Air Mixture,” ASME J. Energy Resour. Technol., 135(2), p. 021001. [CrossRef]
Janbozorgi, M., Sheikhi, M. R. H., and Metghalchi, H., 2013, “Principle of Detailed Balance and the Second Law of Thermodynamics in Chemical Kinetics,” ASME J. Energy Resour. Technol., 135(4), p. 041901. [CrossRef]
Kodama, K., and Kitagawa, K., 2008, “Spectrochemical Analysis in Flames,” J. Japan Spectroscopic Society, 57(2), pp. 69–80. [CrossRef]


Grahic Jump Location
Fig. 1

Typical spectra of laser induced plasma in flame with different targets, (a) Al2O3 and (b) SiO2

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Fig. 2

Atomic emission spectrum in a methane–air diffusion flame with Mg solution using LIPS (at x = 0 mm and z = 15 mm)

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Fig. 3

The Boltzmann plot of Si emission lines

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Fig. 4

Profiles of atomic emission intensity

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Fig. 5

Profiles of emission intensity ratio (normalized by the magnesium intensity)




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